BMOLogo
Publications

LMU München
Fakultät für Physik


Home

General
Research
Funding
Members
Publications
  All Publications
  PhD Theses
  Master Theses
  Search
  i Search
Lectures/Seminars
Conferences
Vacancies
Search

Internal




Impressum
(c) 2002 BMO

"A novel setup for femtosecond pump-repump-probe IR spectroscopy with few cycle CEP stable pulses"
M. Bradler, J. C. Werhahn, D. Hutzler, S. Fuhrmann, R. Heider, E. Riedle, H. Iglev, and R. Kienberger
Opt. Express 21, 20145 - 20158 (2013).


Abstract:
We present a three-color mid-IR setup for vibrational pumprepump-probe experiments with a temporal resolution well below 100 fs and a freely selectable spectral resolution of 20 to 360 cm-1 for the pump and repump. The usable probe range without optical realignment is 900 cm-1. The experimental design employed is greatly simplified compared to the widely used setups, highly robust and includes a novel means for generation of tunable few-cycle pulses with stable carrier-envelope phase. A Ti:sapphire pump system operating with 1 kHz and a modest 150 fs pulse duration supplies the total pump energy of just 0.6 mJ. The good signal-to-noise ratio of the setup allows the determination of spectrally resolved transient probe changes smaller than 6·10-5 OD at 130 time delays in just 45 minutes. The performance of the spectrometer is demonstrated with transient IR spectra and decay curves of HDO molecules in lithium nitrate trihydrate and ice and a first all MIR pump-repump-probe measurement.

BMO authors (in alphabetic order):
Maximilian Bradler
Eberhard Riedle

Order Hardcopy

WWW-Version

mailto: webmaster
Letzte Änderung: 2016-09-14 13:34